The overall aim of the UK Surface Ocean / Lower Atmosphere Study (UK SOLAS) is to advance understanding of environmentally significant interactions between the atmosphere and ocean, focusing on material exchanges that involve ocean productivity, atmospheric composition and climate. The knowledge obtained will improve the predictability of climate change and give insights into the distribution and fate of persistent pollutants. The dataset contains biological and chemical measurements such as: major nutrients and trace metal concentrations in aerosol and rain samples, chemical analyses of inorganic micro-nutrients, dissolved and particulate trace metal and carbon analyses, dissolved nitrogen and organic phosphate, biological measurements including phytoplankton pigments, bacteria, picoplankton and larger phytoplankton abundance.